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N. Alvarado, L. Alegría, C. Sandoval, L. Gargallo, A. Leiva, D. Radic

Synthesis, characterization and molecular dynamics simulation of
dendronized poly(3,5-diphthalimidoalkylphenyl methacrylate)s (in English)

Polimery 2016, No 1, 10

DOI: dx.doi.org/10.14314/polimery.2016.010

Summary
Dendronized methacrylates containing 3,5-diphthalimidoalkylphenyl moieties (with ethyl, propyl or butyl spacer groups) were synthesized. These monomers were then polymerized using radical polymerization. Monomers and polymers were characterized using Fourier transform infrared spectroscopy (FT-IR) and nuclear magnetic resonance methods (¹H NMR and ¹³C NMR). Molecular weight was estimated by multi-angle static light scattering (MALS). Molecular dynamics simulation was performed to evaluate the conformational radius of gyration (R_g) and the end-to-end distance (r_ee). Different spatial arrangements depending on the length of the spacer group are observed.

Keywords: poly(phtalimidoalkyl methacrylate), dendronized polymers, spacer groups, molecular dynamics simulation, radius of gyration, end-to-end distance

e-mail: dradic@puc.cl

N. Alvarado, L. Alegría, C. Sandoval, L. Gargallo, A. Leiva, D. Radic (655.5 KB): Synthesis, characterization and molecular dynamics simulation of dendronized poly(3,5-diphthalimidoalkylphenyl methacrylate)s (in English)